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Improvement of organic solar cells by flexible substrate and ITO surface treatments

Identifieur interne : 003F58 ( Main/Repository ); précédent : 003F57; suivant : 003F59

Improvement of organic solar cells by flexible substrate and ITO surface treatments

Auteurs : RBID : Pascal:10-0412275

Descripteurs français

Pascal (Inist)
- Cellule solaire, Traitement surface, Revêtement dur, Angle contact, Magnétron, Couche mince, Conductivité électrique, Densité porteur charge, Facteur transmission, Structure surface, Travail sortie, Ozone, Densité courant, Oxyde d'indium, Oxyde d'étain, Ethylène téréphtalate polymère, 8460J, 6855J, 7361, 7820C.
Wicri :
- concept : Ozone.

English descriptors

KwdEn :
- Charge carrier density, Contact angle, Current density, Electrical conductivity, Ethylene terephthalate polymer, Hard coating, Indium oxide, Magnetron, Ozone, Solar cell, Surface structure, Surface treatment, Thin film, Tin oxide, Transmittance, Work function.

Abstract

In this paper, surface treatments on polyethylene terephthalate with polymeric hard coating (PET-HC) substrates are described. The effect of the contact angle on the treatment is first investigated. It has been observed that detergent is quite effective in removing organic contamination on the flexible PET-HC substrates. Next, using a DC-reactive magnetron sputter, indium tin oxide (ITO) thin films of90 nm are grown on a substrate treated by detergent. Then, various ITO surface treatments are made for improving the performance of the finally developed organic solar cells with structure Al/P3HT:PCBM/PEDOT:PSS/ITO/PET. It is found that the parameters of the ITO including resistivity, carrier concentration, transmittance, surface morphology, and work function depended on the surface treatments and significantly influence the solar cell performance. With the optimal conditions for detergent treatment on flexible PET substrates, the ITO film with a resistivity of 5.6 x 10^-4Ω cm and average optical transmittance of 84.1% in the visible region are obtained. The optimal ITO surface treated by detergent for 5 min and then by UV ozone for 20 min exhibits the best WF value of 5.22 eV. This improves about 8.30% in the WF compared with that of the untreated ITO film. In the case of optimal treatment with the organic photovoltaic device, meanwhile, 36.6% enhancement in short circuit current density (J_sc) and 92.7% enhancement in conversion efficiency (η) over the untreated solar cell are obtained.

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Le document en format XML

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<author><name sortKey="Cheng, Yuang Tung" uniqKey="Cheng Y">Yuang-Tung Cheng</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Department of Electrical Engineering, National Taiwan Ocean University, No. 2 Pei-ning Rd.</s1>
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<author><name sortKey="Ho, Jyh Jier" uniqKey="Ho J">Jyh-Jier Ho</name>
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<author><name sortKey="Wang, Chien Kun" uniqKey="Wang C">Chien-Kun Wang</name>
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<author><name sortKey="Chang, Shun Hsyung" uniqKey="Chang S">Shun-Hsyung Chang</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Department of Electrical Engineering, National Taiwan Ocean University, No. 2 Pei-ning Rd.</s1>
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<author><name sortKey="Chang, Chiu Cheng" uniqKey="Chang C">Chiu-Cheng Chang</name>
<affiliation wicri:level="1"><inist:fA14 i1="03"><s1>Risk Management Chair Professor, Asia University, 500, Lioufeng Rd.</s1>
<s2>Wufeng, Taichung 41354</s2>
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<author><name sortKey="Wang, Kang L" uniqKey="Wang K">Kang L. Wang</name>
<affiliation wicri:level="1"><inist:fA14 i1="04"><s1>Device Research Lab, Electrical Eng., University of California</s1>
<s2>LA, CA 90095</s2>
<s3>USA</s3>
<sZ>10 aut.</sZ>
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<country>États-Unis</country>
<placeName><region type="state">Louisiane</region>
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<date when="2010">2010</date>
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<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Charge carrier density</term>
<term>Contact angle</term>
<term>Current density</term>
<term>Electrical conductivity</term>
<term>Ethylene terephthalate polymer</term>
<term>Hard coating</term>
<term>Indium oxide</term>
<term>Magnetron</term>
<term>Ozone</term>
<term>Solar cell</term>
<term>Surface structure</term>
<term>Surface treatment</term>
<term>Thin film</term>
<term>Tin oxide</term>
<term>Transmittance</term>
<term>Work function</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Cellule solaire</term>
<term>Traitement surface</term>
<term>Revêtement dur</term>
<term>Angle contact</term>
<term>Magnétron</term>
<term>Couche mince</term>
<term>Conductivité électrique</term>
<term>Densité porteur charge</term>
<term>Facteur transmission</term>
<term>Structure surface</term>
<term>Travail sortie</term>
<term>Ozone</term>
<term>Densité courant</term>
<term>Oxyde d'indium</term>
<term>Oxyde d'étain</term>
<term>Ethylène téréphtalate polymère</term>
<term>8460J</term>
<term>6855J</term>
<term>7361</term>
<term>7820C</term>
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<keywords scheme="Wicri" type="concept" xml:lang="fr"><term>Ozone</term>
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<front><div type="abstract" xml:lang="en">In this paper, surface treatments on polyethylene terephthalate with polymeric hard coating (PET-HC) substrates are described. The effect of the contact angle on the treatment is first investigated. It has been observed that detergent is quite effective in removing organic contamination on the flexible PET-HC substrates. Next, using a DC-reactive magnetron sputter, indium tin oxide (ITO) thin films of90 nm are grown on a substrate treated by detergent. Then, various ITO surface treatments are made for improving the performance of the finally developed organic solar cells with structure Al/P3HT:PCBM/PEDOT:PSS/ITO/PET. It is found that the parameters of the ITO including resistivity, carrier concentration, transmittance, surface morphology, and work function depended on the surface treatments and significantly influence the solar cell performance. With the optimal conditions for detergent treatment on flexible PET substrates, the ITO film with a resistivity of 5.6 x 10<sup>-4 </sup>
Ω cm and average optical transmittance of 84.1% in the visible region are obtained. The optimal ITO surface treated by detergent for 5 min and then by UV ozone for 20 min exhibits the best WF value of 5.22 eV. This improves about 8.30% in the WF compared with that of the untreated ITO film. In the case of optimal treatment with the organic photovoltaic device, meanwhile, 36.6% enhancement in short circuit current density (J<sub>sc</sub>
) and 92.7% enhancement in conversion efficiency (η) over the untreated solar cell are obtained.</div>
</front>
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<fA11 i1="01" i2="1"><s1>CHENG (Yuang-Tung)</s1>
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<fA11 i1="02" i2="1"><s1>HO (Jyh-Jier)</s1>
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<fC01 i1="01" l="ENG"><s0>In this paper, surface treatments on polyethylene terephthalate with polymeric hard coating (PET-HC) substrates are described. The effect of the contact angle on the treatment is first investigated. It has been observed that detergent is quite effective in removing organic contamination on the flexible PET-HC substrates. Next, using a DC-reactive magnetron sputter, indium tin oxide (ITO) thin films of90 nm are grown on a substrate treated by detergent. Then, various ITO surface treatments are made for improving the performance of the finally developed organic solar cells with structure Al/P3HT:PCBM/PEDOT:PSS/ITO/PET. It is found that the parameters of the ITO including resistivity, carrier concentration, transmittance, surface morphology, and work function depended on the surface treatments and significantly influence the solar cell performance. With the optimal conditions for detergent treatment on flexible PET substrates, the ITO film with a resistivity of 5.6 x 10<sup>-4 </sup>
Ω cm and average optical transmittance of 84.1% in the visible region are obtained. The optimal ITO surface treated by detergent for 5 min and then by UV ozone for 20 min exhibits the best WF value of 5.22 eV. This improves about 8.30% in the WF compared with that of the untreated ITO film. In the case of optimal treatment with the organic photovoltaic device, meanwhile, 36.6% enhancement in short circuit current density (J<sub>sc</sub>
) and 92.7% enhancement in conversion efficiency (η) over the untreated solar cell are obtained.</s0>
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<s5>01</s5>
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<s5>01</s5>
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<s5>01</s5>
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<s5>02</s5>
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<s5>02</s5>
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<s5>03</s5>
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<s5>03</s5>
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<s5>03</s5>
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<s5>04</s5>
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<s5>04</s5>
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<s5>04</s5>
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<s5>05</s5>
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<s5>05</s5>
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<s5>05</s5>
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<s5>09</s5>
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<s5>09</s5>
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<s5>09</s5>
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<s5>11</s5>
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<s5>11</s5>
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<s5>12</s5>
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<s5>12</s5>
</fC03>
<fC03 i1="08" i2="X" l="SPA"><s0>Concentración portador carga</s0>
<s5>12</s5>
</fC03>
<fC03 i1="09" i2="X" l="FRE"><s0>Facteur transmission</s0>
<s5>13</s5>
</fC03>
<fC03 i1="09" i2="X" l="ENG"><s0>Transmittance</s0>
<s5>13</s5>
</fC03>
<fC03 i1="09" i2="X" l="SPA"><s0>Factor transmisión</s0>
<s5>13</s5>
</fC03>
<fC03 i1="10" i2="X" l="FRE"><s0>Structure surface</s0>
<s5>14</s5>
</fC03>
<fC03 i1="10" i2="X" l="ENG"><s0>Surface structure</s0>
<s5>14</s5>
</fC03>
<fC03 i1="10" i2="X" l="SPA"><s0>Estructura superficie</s0>
<s5>14</s5>
</fC03>
<fC03 i1="11" i2="X" l="FRE"><s0>Travail sortie</s0>
<s5>15</s5>
</fC03>
<fC03 i1="11" i2="X" l="ENG"><s0>Work function</s0>
<s5>15</s5>
</fC03>
<fC03 i1="11" i2="X" l="SPA"><s0>Función de trabajo</s0>
<s5>15</s5>
</fC03>
<fC03 i1="12" i2="X" l="FRE"><s0>Ozone</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>16</s5>
</fC03>
<fC03 i1="12" i2="X" l="ENG"><s0>Ozone</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>16</s5>
</fC03>
<fC03 i1="12" i2="X" l="SPA"><s0>Ozono</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>16</s5>
</fC03>
<fC03 i1="13" i2="X" l="FRE"><s0>Densité courant</s0>
<s5>17</s5>
</fC03>
<fC03 i1="13" i2="X" l="ENG"><s0>Current density</s0>
<s5>17</s5>
</fC03>
<fC03 i1="13" i2="X" l="SPA"><s0>Densidad corriente</s0>
<s5>17</s5>
</fC03>
<fC03 i1="14" i2="X" l="FRE"><s0>Oxyde d'indium</s0>
<s5>18</s5>
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<fC03 i1="14" i2="X" l="ENG"><s0>Indium oxide</s0>
<s5>18</s5>
</fC03>
<fC03 i1="14" i2="X" l="SPA"><s0>Indio óxido</s0>
<s5>18</s5>
</fC03>
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<s5>19</s5>
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<fC03 i1="15" i2="X" l="ENG"><s0>Tin oxide</s0>
<s5>19</s5>
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<fC03 i1="15" i2="X" l="SPA"><s0>Estaño óxido</s0>
<s5>19</s5>
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<fC03 i1="16" i2="X" l="FRE"><s0>Ethylène téréphtalate polymère</s0>
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<s5>22</s5>
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<fC03 i1="16" i2="X" l="ENG"><s0>Ethylene terephthalate polymer</s0>
<s2>NK</s2>
<s5>22</s5>
</fC03>
<fC03 i1="16" i2="X" l="SPA"><s0>Etileno tereftalato polímero</s0>
<s2>NK</s2>
<s5>22</s5>
</fC03>
<fC03 i1="17" i2="X" l="FRE"><s0>8460J</s0>
<s2>PAC</s2>
<s4>INC</s4>
<s5>45</s5>
</fC03>
<fC03 i1="18" i2="X" l="FRE"><s0>6855J</s0>
<s2>PAC</s2>
<s4>INC</s4>
<s5>46</s5>
</fC03>
<fC03 i1="19" i2="X" l="FRE"><s0>7361</s0>
<s2>PAC</s2>
<s4>INC</s4>
<s5>47</s5>
</fC03>
<fC03 i1="20" i2="X" l="FRE"><s0>7820C</s0>
<s2>PAC</s2>
<s4>INC</s4>
<s5>48</s5>
</fC03>
<fC07 i1="01" i2="X" l="FRE"><s0>Composé minéral</s0>
<s5>07</s5>
</fC07>
<fC07 i1="01" i2="X" l="ENG"><s0>Inorganic compound</s0>
<s5>07</s5>
</fC07>
<fC07 i1="01" i2="X" l="SPA"><s0>Compuesto inorgánico</s0>
<s5>07</s5>
</fC07>
<fC07 i1="02" i2="3" l="FRE"><s0>Composé de métal de transition</s0>
<s5>08</s5>
</fC07>
<fC07 i1="02" i2="3" l="ENG"><s0>Transition element compounds</s0>
<s5>08</s5>
</fC07>
<fN21><s1>270</s1>
</fN21>
</pA>
</standard>
</inist>
</record>

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Improvement of organic solar cells by flexible substrate and ITO surface treatments

Improvement of organic solar cells by flexible substrate and ITO surface treatments

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